journal article·2026-07-14Open access

Rational Design of Hydrocarbon Proton-Conducting Membranes Replacing Perfluorosulfonic Acids in Polymer Electrolyte Membrane Water Electrolysis

Giorgi Titvinidze, Nodar Dumbadze, Jules-Fabien Kreuer, Carolin Klose, Andreas Münchinger, Clara Schare, Barbara Heck, Christina Oeß, Michael Schuster, David Hicke, Klaus-Dieter Kreuer

Chemistry of Materials· Volume 38· Issue 13

Abstract

High Resolution Image Download MS PowerPoint Slide Contrasting the characteristic properties of PFSAs such as Nafion and hydrocarbon membranes suggests that PEM water electrolysis could become a first showcase for the competitive use of hydrocarbon membranes. The main reasons are high proton conductivity and low hydrogen permeability of many sulfonated polyarylenes and phenylenes under water electrolysis conditions. Within this class of ionomers, we have, therefore, downselected according to thermohydrolytic stability, a conditio sine qua non for the use of membranes in PEM electrolyzers. We identified the family of sulfonated poly(phenylene sulfones) (sPPS) as virtually inert hydrocarbon ionomers. The remaining critical issues of sPPS membranes, especially exaggerated swelling at high ion exchange capacity, softening in hot water ( T = 80 °C) and fatigue under wet/dry cycling conditions, were significantly mitigated by (i) introducing into the homogeneously (ordered) sulfonated polymer structure uniform unsulfonated segments aggregating into well-connected networks counterbalancing osmotic pressure and (ii) introducing ductile polyethylene nanoporous reinforcements serving as fracture toughener. The present rational design approach provided the basis for successful in situ electrolyzer tests of 24 μm thick sPPS-based membranes published in a separate paper. This features lower ohmic losses along with a more than 2-fold reduced hydrogen crossover compared to Nafion 211 and stable operation over 2000 h at a current density of 1 A cm –2 without failure to the end of the test.
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Research context

OpenAlex topics: Fuel Cells and Related Materials · Membrane-based Ion Separation Techniques · Hybrid Renewable Energy Systems

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Laboratory of Engineering Polymers, Agricultural University of Georgia, 240 David Aghmashenebeli Alley, 0131 Tbilisi, Georgia

Hahn-Schickard, Georges-Koehler-Allee 103, 79110 Freiburg, Germany

Eberhard-Karls-Universität Tübingen

Electrochemical Energy Systems, IMTEK─Department of Microsystems Engineering, University of Freiburg, Georges-Koehler-Allee 103, 79110 Freiburg, Germany

Institute of Physics, University of Freiburg, Hermann-Herder-Str. 3, 79104 Freiburg, Germany

Institute of Energy Technologies─Fundamental Electrochemistry (IET-1), Forschungszentrum Jülich GmbH, Wilhelm-Johnen-Straße, 52425 Jülich, Germany

Institute of Physical Chemistry

RWTH Aachen University

FUMATECH BWT GmbH, Carl-Benz-Straße 4, 74321 Bietigheim-Bissingen, Germany

Max Planck Institute for Solid State Research, Heisenbergstraße 1, 70569 Stuttgart, Germany

Funding

Bundesministerium f?r Bildung und Forschung · Shota Rustaveli National Science Foundation · Volkswagen Foundation

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