journal article·2022-03-17

Interplay between Charge-Density-Wave, Superconductivity, and Ferromagnetism in CuIr2–xCrxTe4 Chalcogenides

Lingyong Zeng, Xunwu Hu, Ningning Wang, Jianping Sun, Pengtao Yang, Mebrouka Boubeche, Shaojuan Luo, Yiyi He, Jinguang Cheng, Dao-Xin Yao, Huixia Luo

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Abstract

We report the crystal structure, charge-density-wave (CDW), superconductivity (SC), and ferromagnetism (FM) in CuIr 2– x Cr x Te 4 (0 ≤ x ≤ 2) chalcogenides. Powder x-ray diffraction (PXRD) results reveal that the CuIr 2– x Cr x Te 4 series are distinguished between two structural types and three different regions: (i) layered trigonal structure region, (ii) mixed phase regions, and (iii) spinel structure region. Besides, Cr substitution for Ir site results in rich physical properties including the collapse of CDW, the formation of dome-shaped like SC, and the emergence of magnetism. Cr doping slightly elevates the superconducting critical temperature ( T sc ) to its highest T sc = 2.9 K around x = 0.06. As x increases from 0.3 to 0.4, the ferromagnetic Curie temperature ( T c ) increases from 175 to 260 K. However, the T c remains unchanged in the spinel range of 1.9 ≤ x ≤ 2. This finding provides a comprehensive material platform for investigating the interplay between CDW, SC, and FM multipartite quantum states.
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Research context

OpenAlex topics: Iron-based superconductors research · Rare-earth and actinide compounds · Advanced Condensed Matter Physics

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Affiliations

School of Materials Science and Engineering, State Key Laboratory of Optoelectronic Materials and Technologies, Key Lab of Polymer Composite & Functional Materials, Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices, Sun Yat-Sen University, No. 135, Xingang Xi Road, Guangzhou, 510275, P. R. China

School of Physics, Center for Neutron Science and Technology, State Key Laboratory of Optoelectronic Materials and Technologies, Sun Yat-Sen University, Guangzhou, 510275, P. R. China

Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences and School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100190, P. R. China

School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou, 510006, P. R. China

Funding

Ministry of Science and Technology of the People's Republic of China · Central University Basic Research Fund of China · National Natural Science Foundation of China · Guangdong Province · Guangdong Basic and Applied Basic Research Foundation

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