journal article·2024-11-14

Transferable and Interpretable Prediction of Site-Specific Dehydrogenation Reaction Rate Constants with NMR Spectra

Yanbo Li, Fenfen Ma, Zhandong Wang, Xin Chen

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Abstract

Accurate and efficient determination of site-specific reaction rate constants over a wide temperature range remains challenging, both experimentally and theoretically. Taking the dehydrogenation reaction as an example, our study addresses this issue by an innovative combination of machine learning techniques and cost-effective NMR spectra. Through descriptor screening, we identified a minimal set of NMR chemical shifts that can effectively determine reaction rate constants. The constructed model performs exceptionally well on theoretical data sets and demonstrates impressive generalization capabilities, extending from small molecules to larger ones. Furthermore, this model shows outstanding performance when applied to limited experimental data sets, highlighting its robust applicability and transferability. Utilizing the Sure Independence Screening and Sparsifying Operator (SISSO) algorithm, we also present an interpretable rate constant-temperature-NMR (k-T-NMR) relationship with a mathematical formula. This study reveals the great potential of combining machine learning with easily accessible spectroscopic descriptors in the study of reaction kinetics, enabling the rapid determination of reaction rate constants and promoting our understanding of reactivity.
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Research context

OpenAlex topics: Metabolomics and Mass Spectrometry Studies · Machine Learning in Materials Science · NMR spectroscopy and applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China

GuSu Laboratory of Materials, Suzhou 215123, China

National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, China

Suzhou Laboratory, Suzhou 215123, China

Funding

National Key Research and Development Program of China

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