Simulating Asymmetric Top Impurities in Superfluid Clusters: A para-Water Dopant in para-Hydrogen
Source abstract
Abstract
We present the first simulation study of bosonic clusters doped with an asymmetric top molecule. The path-integral Monte Carlo method with the latest methodological advance in treating rigid-body rotation [Noya, E. G.; Vega, C.; McBride, C. J. Chem. Phys.2011, 134, 054117] is employed to study a para-water impurity in para-hydrogen clusters with up to 20 para-hydrogen molecules. The growth pattern of the doped clusters is similar in nature to that of pure clusters. The para-water molecule appears to rotate freely in the cluster. The presence of para-water substantially quenches the superfluid response of para-hydrogen with respect to the space-fixed frame.
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Research context
OpenAlex topics: Quantum, superfluid, helium dynamics · Cold Atom Physics and Bose-Einstein Condensates · Physics of Superconductivity and Magnetism
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Department of Chemistry, University of Waterloo, Waterloo, ON N2L 3G1, Canada
Institute of Theoretical Chemistry, State Key Laboratory of Theoretical and Computational Chemistry, Jilin University, 2519 Jiefang Road, Changchun 130023, People’s Republic of China
References (38)
Show source-provided references
1. Ginsburg L. · JETP Lett. · 1972 · 15 · 242
2. Sindzingre P. · Phys. Rev. Lett. · 1991 · 67 · 187110.1103/PhysRevLett.67.1871 ↗
3. Grebenev S. · Science · 2000 · 289 · 153210.1126/science.289.5484.1532 ↗
4. Grebenev S. · Phys. Rev. Lett. · 2002 · 89 · 22530110.1103/PhysRevLett.89.225301 ↗
5. Paesani F. · J. Chem. Phys. · 2005 · 122 · 18110610.1063/1.1913552 ↗
6. Paesani F. · J. Chem. Phys. · 2003 · 119 · 1168210.1063/1.1624058 ↗
7. Kwon Y. · Phys. Rev. Lett. · 2002 · 89 · 27340110.1103/PhysRevLett.89.273401 ↗
8. Moore D. · J. Chem. Phys. · 2003 · 119 · 471310.1063/1.1590639 ↗
9. Moore D. T. · J. Phys. Chem. A · 2003 · 107 · 1080510.1021/jp0306343 ↗
10. Moore D. T. · J. Phys. Chem. A · 2004 · 108 · 193010.1021/jp0310403 ↗
11. Kwon Y. · J. Low Temp. Phys. · 2005 · 140 · 277
12. Piccarreta C. · Eur. Phys. J. D · 2006 · 37 · 9310.1140/epjd/e2005-00245-y ↗
13. Grebenev S. · Europhys. Lett. · 2008 · 83 · 6600810.1209/0295-5075/83/66008 ↗
14. Grebenev S. · J. Chem. Phys. · 2010 · 132 · 06450110.1063/1.3274509 ↗
15. Li H. · Phys. Rev. Lett. · 2010 · 105 · 13340110.1103/PhysRevLett.105.133401 ↗
16. de Lara-Castells M. P. · J. Phys. Chem. Lett. · 2011 · 2 · 214510.1021/jz200801r ↗
17. Raston P. L. · Phys. Rev. Lett. · 2012 · 108 · 25340210.1103/PhysRevLett.108.253402 ↗
18. Lee E. · Phys. Rev. Lett. · 1999 · 83 · 381210.1103/PhysRevLett.83.3812 ↗
19. Markovskiy N. D. · J. Phys. Chem. A · 2009 · 113 · 916510.1021/jp900718d ↗
20. Noya E. G. · J. Chem. Phys. · 2011 · 134 · 05411710.1063/1.3544214 ↗
21. Moroni S. · J. Chem. Phys. · 2004 · 121 · 357710.1063/1.1774160 ↗
22. Blinov N. · J. Low. Temp. Phys. · 2005 · 140 · 25310.1007/s10909-005-6312-y ↗
23. Li H. · J. Chem. Phys. · 2009 · 130 · 14430510.1063/1.3109897 ↗
24. Boninsegni M. · Phys. Rev. Lett. · 2006 · 96 · 07060110.1103/PhysRevLett.96.070601 ↗
25. Boninsegni M. · Phys. Rev. E · 2006 · 74 · 03670110.1103/PhysRevE.74.036701 ↗
26. Patkowski K. · J. Chem. Phys. · 2008 · 129 · 09430410.1063/1.2975220 ↗
27. Zeng T. · J. Chem. Phys. · 2011 · 135 · 09430410.1063/1.3626840 ↗
28. Knuth E. · J. Chem. Phys. · 1995 · 102 · 628510.1063/1.469072 ↗
29. Humphrey W. · J. Molec. Graphics · 1996 · 14 · 3310.1016/0263-7855(96)00018-5 ↗
30. Khairallah S. A. · Phys. Rev. Lett. · 2007 · 98 · 18340110.1103/PhysRevLett.98.183401 ↗
31. Blinov N. · J. Chem. Phys. · 2004 · 120 · 591610.1063/1.1650301 ↗
32. Ceponkus J. · J. Phys. Chem. A · 2010 · 114 · 1297910.1021/jp105303z ↗
33. Ceponkus J. · J. Phys. Chem. A · 2011 · 115 · 792110.1021/jp201751r ↗
34. Ceperley D. M. · Rev. Mod. Phys. · 1995 · 67 · 27910.1103/RevModPhys.67.279 ↗
35. Suárez A. G. · Chem. Phys. Lett. · 2011 · 502 · 1410.1016/j.cplett.2010.12.006 ↗
36. Andronikashvili E. · J. Phys. USSR · 1946 · 10 · 201
37. Mezzacapo F. · J. Phys.: Condens. Matter · 2009 · 21 · 164205
38. Mezzacapo F. · Phys. Rev. Lett. · 2008 · 100 · 14530110.1103/PhysRevLett.100.145301 ↗